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Ammonia-assisted fast Li-ion conductivity in a new hemiammine lithium borohydride,LiBH4 center dot 1/2NH(3)

Author:
Yan, Yigang  Grinderslev, Jakob B.  Lee, Young-Su  Jorgensen, Mathias  Cho, Young Whan  Cerny, Radovan  Jensen, Torben R.  


Journal:
CHEMICAL COMMUNICATIONS


Issue Date:
2020


Abstract(summary):

Hemiammine lithium borohydride, LiBH4 center dot 1/2NH(3), is characterized and a new Li+ conductivity mechanism is identified. It exhibits a Li+ conductivity of 7 x 10(-4) S cm(-1) at 40 degrees C in the solid state and 3.0 x 10(-2) S cm(-1) at 55 degrees C after melting. The molten state of LiBH4 center dot 1/2NH(3) has a high viscosity and can be mechanically stabilized in nano-composites with inert metal oxides and other hydrides making it a promising battery electrolyte.


Page:
3971---3974


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