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Low-temperature properties of pyrochlore Lu2Ir2O7

Author:
Klicpera, M.  Vlaskova, K.  Divis, M.  


Journal:
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS


Issue Date:
2020


Abstract(summary):

Low-temperature properties of Lu2Ir2O7 were studied by means of magnetization, ac-susceptibility and specific heat measurements. Our low-temperature measurements reveal a bifurcation of ZFC and FC magnetization data below 140 K, which is further pronounced as a broad anomaly in the temperature development of specific heat and ac-susceptibility. The anomaly can be attributed to the same physical mechanism as discussed for other A(2)Ir(2)O(7) with A =3D magnetic rare-earth element, i.e. to short-range correlations among Ir-4(+) magnetic moments, rather than to a long-range order of Ir sublattice reported earlier. The ac-susceptibility data revealed a strong frequency dependence of the signal, a paradigmatic sign of a spin-glass transition. The analysis of low-temperature specific heat data brought important information on physical properties of Lu2Ir2O7, in striking agreement with our density functional theoretical (DFT) calculations, concluding relatively weak electron-phonon interaction and semimetallic ground state in Lu2Ir2O7.


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