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On the general mechanism of photocatalytic reduction of CO2

Author:
Elham Karamian  Shahram Sharifnia  


Journal:
Journal of CO2 Utilization


Issue Date:
2016


Abstract(summary):

Abstract This paper is going to make a global view of the reaction mechanism of photocatalytic reduction of CO 2 . During the past decades, extensive studies have been conducted to identify the photocatalytic products of CO 2 conversion and their reaction mechanisms. There is a need to propose a general mechanism pattern covering the results of these original researches. Among many factors affecting the redox reaction pathway, this paper focuses on the effect of reductant type as an important issue on the product diversity and selectivity of CO 2 photocatalysis. We first tried to show the reaction mechanism of CO 2 photocatalysis in the solitary presence of the most common reductants, H 2 , H 2 O (both gaseous and aqueous phases), CH 4 , and CH 3 OH. Then, a general mechanism has been suggested for CO 2 conversion in the mixture of the reductants, based on the fact that in the photoreduction process of CO 2 , all of the reductants can be derived from one of them.


Page:
194-194


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