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Total Syntheses of (+/-)-Rhodonoids C,D,E,F,and G and Ranhuadujuanine B

Author:
Wu, Hao  Hsung, Richard P.  Tang, Yu  


Journal:
ORGANIC LETTERS


Issue Date:
2017


Abstract(summary):

Here we describe the divergent, biosynthetically inspired syntheses of (+/-)-rhodonoids C-G and (+/-)-ranhuadujuanine B. The key steps of the Syntheses inelude the construction: of the chromene unit through a formal oxa-[3 + 3] annulation and a biomimetic acid-catalyzed ring Cyclization. Cationic [2 + 2]:cydoadclition is accomplished to form the cyclobutane core of (+/-)-rhcidonoids E and F.


Page:
3505---3507


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